The top cancer success stories of the past 50 years, by the numbers
Heidi Ledford
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共 12 篇,分为 4 组
Heidi Ledford
Ewen Callaway
Ewen Callaway
Chris Stokel-Walker
Saskia Popescu
Flora Graham
Jacob Smith
Naihao Ye
Xiaobo Ji
Steven Wang
Xu Hou
Junwang Tang
Abstract Catalytic hydrogen production from methanol offers a promising green route for safe and convenient hydrogen storage and transport and on-demand generation but remains challenging. Here we report a modulated single-atom-based catalytic cluster, assisted by a photon–phonon co-driven strategy, capable of achieving efficient hydrogen production from methanol solution with co-generation of green formaldehyde. By stabilizing Pt single atoms on TiO 2 surface through Li-modulated microenvironments, the PtLi 2 cluster-immobilized TiO 2 catalyst achieves an exceptional hydrogen production rate of 4.36 mol g −1 h −1 at 150 °C, corresponding to an overall quantum yield as high as 184%. Furthermore, a 21.2 wt% concentrated formaldehyde solution is synthesized, offering a potential commercial…